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. Supramolecular ring-in-ring sandwich nanotransporters for controlled and synchronized release of multiple cargos. We report a supramolecular ring-in-ring (SIR) nanotransporter comprising a polyether-based hydrogel and a cationic peptide amphiphile, which self-assembles in water into nanotransporters with a ring-in-ring architecture. The gel layer segregates the hydrophobic cargo from the aqueous solution and the cationic peptide provides self-aggregation and self-healing properties. The cargo release is tuned by manipulating the hydrogel permeability and the gel concentration. The SIR nanotransporter can simultaneously deliver two different cargos with different release rates. We demonstrate that these nanotransporters can be used to package and release multiple payloads and use multiple cargo release strategies, simultaneously releasing these multiple cargos in a synchronized manner and with controlled release rates.

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